Find the account that logged on in a way it never should
Group every successful logon by its Logon Type and count them. One type accounts for the overwhelming majority, which is a file server doing its job; the uncommon types are where to look, and logon-types.md explains what kind of access each one represents. List the accounts behind each uncommon type, then cross-reference asset-inventory.csv, which records host ownership and what each registered account is approved to do. Most of those accounts are doing something approved, so the type on its own gives you a shortlist and not a finding: the finding is the account for which that kind of logon is not an approved use at all.